Phase-only shaped laser pulses in optimal control theory: application to indirect photofragmentation dynamics in the weak-field limit.
نویسندگان
چکیده
We implement phase-only shaped laser pulses within quantum optimal control theory for laser-molecule interaction. This approach is applied to the indirect photofragmentation dynamics of NaI in the weak-field limit. It is shown that optimized phase-modulated pulses with a fixed frequency distribution can substantially modify transient dissociation probabilities as well as the momentum distribution associated with the relative motion of Na and I.
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عنوان ژورنال:
- The Journal of chemical physics
دوره 136 4 شماره
صفحات -
تاریخ انتشار 2012